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Chemical probe systems for assessing liquid–liquid mixing efficiencies of reactors

《化学科学与工程前沿（英文）》 2023年 第17卷 第10期   页码 1323-1335 doi: 10.1007/s11705-022-2275-7

摘要： Liquid–liquid mixing, including homogeneous and heterogeneous mixing, widely exists in the chemical industry. How to quantitatively characterize the mixing performance is important for reactor assessment and development. As a convenient and direct method for mixing characterization, the chemical probe method uses some special test reactions to characterize the mixing results. Here, the working principle and selection requirements of this method are introduced, and some common chemical probe systems for homogeneous and heterogeneous mixing processes are reviewed. The characteristics and applications of these systems are illustrated. Finally, the development of the new system is proposed.

关键词： mixing     chemical probe     liquid–liquid     heterogeneous    

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Energy-aware scheduling with reconstruction and frequency equalization on heterogeneous systems

Yong-xing LIU,Ken-li LI,Zhuo TANG,Ke-qin LI

《信息与电子工程前沿（英文）》 2015年 第16卷 第7期   页码 519-531 doi: 10.1631/FITEE.1400399

摘要： With the increasing energy consumption of computing systems and the growing advocacy for green computing, energy efficiency has become one of the critical challenges in high-performance heterogeneous computing systems. Energy consumption can be reduced by not only hardware design but also software design. In this paper, we propose an energy-aware scheduling algorithm with equalized frequency, called EASEF, for parallel applications on heterogeneous computing systems. The EASEF approach aims to minimize the finish time and overall energy consumption. First, EASEF extracts the set of paths from an application. Then, it reconstructs the application based on the extracted set of paths to achieve a reasonable schedule. Finally, it adopts a progressive way to equalize the frequency of tasks to reduce the total energy consumption of systems. Randomly generated applications and two real-world applications are examined in our experiments. Experimental results show that the EASEF algorithm outperforms two existing algorithms in terms of makespan and energy consumption.

关键词： Directed acyclic graph     Dynamic voltage scaling     Energy aware     Heterogeneous systems     Task scheduling    

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基于分布式事件触发策略的异构非线性多智能体系统包含控制 Research Articles

孙雅妮,邹文成,郭健,向峥嵘

《信息与电子工程前沿（英文）》 2021年 第22卷 第1期   页码 1-140 doi: 10.1631/FITEE.2000034

摘要： 研究分布式事件触发策略下高阶异构非线性多智能体系统包含控制问题。为实现包含控制目标并减少智能体间的通讯损耗，采用反推控制法、李雅普诺夫函数分析法和神经网络，提出一种分布式事件触发控制策略。为避免对状态误差的连续监测，将事件触发情形的结论推广到自触发控制情形。所提控制协议和触发规则确保每个智能体的输出能在一定误差范围内收敛到有多个领导者信号组成的凸包中。此外，所有智能体都不会发生Zeno现象。最后，通过两个数值仿真案例证明所得结论的正确性。

关键词： 多智能体系统；分布式事件触发控制；包含控制；异构非线性系统；Zeno现象    

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针对异构隐式反馈的置信度估计方法 Article

Jing WANG, Lan-fen LIN, Heng ZHANG, Jia-qi TU, Peng-hua YU

《信息与电子工程前沿（英文）》 2017年 第18卷 第11期   页码 1817-1827 doi: 10.1631/FITEE.1601468

摘要： 隐式反馈是指用户通过行为间接表达用户的意见。由于其在现实世界中的易得性和丰富性，越来越受到推荐系统领域的关注。使用隐式反馈的常见做法是把隐式反馈当做正面或者负面的用户偏好，并附带不同的置信度。这类方法大多认为，与隐式反馈相关的数值（例如观看的时间）反映了置信度的大小，并且数值越大代表置信度越大。这种假设只适合只有一种隐式反馈的场景。然而在现实世界中，经常同时存在多种隐式反馈，称为异构隐式反馈。现有方法无法有效地从异构隐式反馈中推测出置信度。本文提出了一种新颖的利用异构隐式反馈预测置信度的方法，把预测的置信度应用到“基于点的”和“基于对的”矩阵分解模型中，并提出了一种更通用的方法来为“基于对的”方法选择有效的训练样本。在天猫提供的真实电商数据集上的实验表明，本文方法在多个指标上的效果均要优于现有的方法。

关键词： 推荐系统；异构隐式反馈；置信度；协同过滤；电商    

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Computational design of heterogeneous catalysts and gas separation materials for advanced chemical processing

Huaiwei Shi, Teng Zhou

《化学科学与工程前沿（英文）》 2021年 第15卷 第1期   页码 49-59 doi: 10.1007/s11705-020-1959-0

摘要： Functional materials are widely used in chemical industry in order to reduce the process cost while simultaneously increase the product quality. Considering their significant effects, systematic methods for the optimal selection and design of materials are essential. The conventional synthesis-and-test method for materials development is inefficient and costly. Additionally, the performance of the resulting materials is usually limited by the designer’s expertise. During the past few decades, computational methods have been significantly developed and they now become a very important tool for the optimal design of functional materials for various chemical processes. This article selectively focuses on two important process functional materials, namely heterogeneous catalyst and gas separation agent. Theoretical methods and representative works for computational screening and design of these materials are reviewed.

关键词： heterogeneous catalyst     gas separation     solvent     porous adsorbent     material screening and design    

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Application of heterogeneous catalysis to biodiesel synthesis using microalgae oil

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1343-9

摘要：

• Microalgae oil application for biodiesel synthesis is discussed.

关键词： Biodiesel     Heterogeneous catalysis     Transesterification     Microalgae oil    

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Undrained seismic bearing capacity of strip footing adjacent to a heterogeneous excavation

《结构与土木工程前沿（英文）》 2023年 第17卷 第4期   页码 566-583 doi: 10.1007/s11709-023-0905-x

摘要： The analysis of the bearing capacity of strip footings sited near an excavation is critical in geotechnics. In this study, the effects of the geometrical features of the excavation and the soil strength properties on the seismic bearing capacity of a strip footing resting on an excavation were evaluated using the lower and upper bounds of the finite element limit analysis method. The effects of the setback distance ratio (L/B), excavation height ratio (H/B), soil strength heterogeneity (kB/cu), and horizontal earthquake coefficient (kh) were analyzed. Design charts and tables were produced to clarify the relationship between the undrained seismic bearing capacity and the selected parameters.

关键词： excavation     finite element limit analysis     heterogeneous soil     strip footing     undrained bearing capacity    

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Precursor-driven structural tailoring of iron oxychloride for enhanced heterogeneous Fenton activity

《化学科学与工程前沿（英文）》 2023年 第17卷 第10期   页码 1533-1543 doi: 10.1007/s11705-023-2330-z

摘要： Iron oxychloride (FeOCl) is a unique layered material with tunable electronic properties. The conventional synthetic route of chemical vapor transition involves a thermodynamics-driven gas–solid interfacial reaction which often generates macroscopic crystals with stable facets. In this study, through analyzing the effects of the synthetic parameters on the FeOCl synthesis, we discovered the dominant contribution of the α-Fe2O3 precursors on the chemical property of the FeOCl product, and subsequently developed a highly-controllable synthetic route of tailoring the FeOCl structures into small sizes and exposed high-energy facets via a facile and scalable mechanical-chemical approach. The synthesized products could be systematically tuned by the ball-milling conditions of the α-Fe2O3 precursors. With increased milling time, the FeOCl crystallites demonstrated reduced sizes and more exposed (110) facets. Intriguingly, these small-sized FeOCl catalysts exhibited much faster Fenton-like kinetics than the pristine macroscopic FeOCl materials. Specifically, FeOCl catalysts with a 12-hour milling time showed nearly 39 times higher efficiency toward phenol degradation than the pristine FeOCl. The structure-reactivity relationship was further elucidated using the combinatory analysis via density functional theory calculation, electron paramagnetic resonance and radical quenching probe experiments. This work provides a rationale for tailoring the surface structures of FeOCl crystallites for potential applications in environmental catalysis.

关键词： FeOCl     mechanical activation     heterogeneous Fenton reaction     ball milling    

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of herding behavior of tradable green certificate market players on market efficiency: Insights from heterogeneous

《能源前沿（英文）》 2023年 第17卷 第2期   页码 266-285 doi: 10.1007/s11708-021-0752-1

摘要： Tradable green certificate (TGC) scheme promotes the development of renewable energy industry which currently has a dual effect on economy and environment. TGC market efficiency is reflected in stimulating renewable energy investment, but may be reduced by the herding behavior of market players. This paper proposes and simulates an artificial TGC market model which contains heterogeneous agents, communication structure, and regulatory rules to explore the characteristics of herding behavior and its effects on market efficiency. The results show that the evolution of herding behavior reduces information asymmetry and improves market efficiency, especially when the borrowing is allowed. In addition, the fundamental strategy is diffused by herding evolution, but TGC market efficiency may be remarkably reduced by herding with borrowing mechanism. Moreover, the herding behavior may evolve to an equilibrium where the revenue of market players is comparable, thus the fairness in TGC market is improved.

关键词： tradable green certificate     herding behavior     evolution     heterogeneous agent model     complex network    

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Using heterogeneous patent network features to rank and discover influential inventors

Yong-ping DU,Chang-qing YAO,Nan LI

《信息与电子工程前沿（英文）》 2015年 第16卷 第7期   页码 568-578 doi: 10.1631/FITEE.1400394

摘要： Most classic network entity sorting algorithms are implemented in a homogeneous network, and they are not applicable to a heterogeneous network. Registered patent history data denotes the innovations and the achievements in different research fields. In this paper, we present an iteration algorithm called inventor-ranking, to sort the influences of patent inventors in heterogeneous networks constructed based on their patent data. This approach is a flexible rule-based method, making full use of the features of network topology. We sort the inventors and patents by a set of rules, and the algorithm iterates continuously until it meets a certain convergence condition. We also give a detailed analysis of influential inventor’s interesting topics using a latent Dirichlet allocation (LDA) model. Compared with the traditional methods such as PageRank, our approach takes full advantage of the information in the heterogeneous network, including the relationship between inventors and the relationship between the inventor and the patent. Experimental results show that our method can effectively identify the inventors with high influence in patent data, and that it converges faster than PageRank.

关键词： Heterogeneous patent network     Influence     Rule-based ranking    

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Elastic analysis of heterogeneous thick-walled spherical pressure vessels with parabolic varying properties

Keyhan KARAMI, Majid ABEDI, Mohammad ZAMANI NEJAD, Mohammad Hassan LOTFIAN

《机械工程前沿（英文）》 2012年 第7卷 第4期   页码 433-438 doi: 10.1007/s11465-012-0336-1

摘要：

On the basis of plane elasticity theory (PET), the displacement and stress components in a thick-walled spherical pressure vessels made of heterogeneous materials subjected to internal and external pressure is developed. The mechanical properties except the Poisson’s ratio are assumed to obey the parabolic variations throughout the thickness. Effect of material inhomogeneity on the elastic deformations and stresses is investigated. The analytical solutions and the solutions carried out through the FEM have a good agreement. The values used in this study are arbitrary chosen to demonstrate the effect of inhomogeneity on displacements, and stresses distributions.

关键词： thick-walled spherical vessels     heterogeneous materials     FGM     FEM     parabolic varying properties    

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Enhanced heterogeneous Fenton-like activity by Cu-doped BiFeO

Jie Mao, Xie Quan, Jing Wang, Cong Gao, Shuo Chen, Hongtao Yu, Yaobin Zhang

《环境科学与工程前沿（英文）》 2018年 第12卷 第6期 doi: 10.1007/s11783-018-1060-9

摘要：

OH played a key role in heterogeneous Fenton-like catalytic oxidation of organic pollutants.

Doping Cu into BiFeO3 promoted the generation of Fe2+ and then facilitated the effective formation of •OH.

Cu-doped BiFeO3 exhibited higher catalytic performance for phenol degradation than non-doped BiFeO3.

关键词： Cu doped BiFeO3     Heterogeneous Fenton-like catalysts     Oxidative degradation    

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Fe-Mn-sepiolite as an effective heterogeneous Fenton-like catalyst for the decolorization of reactive

Chengyuan SU,Weiguang LI,Xingzhe LIU,Xiaofei HUANG,Xiaodan YU

《环境科学与工程前沿（英文）》 2016年 第10卷 第1期   页码 37-45 doi: 10.1007/s11783-014-0729-y

摘要： A study of the decolorization of reactive brilliant blue in an aqueous solution using Fe-Mn-sepiolite as a heterogeneous Fenton-like catalyst has been performed. The Fourier transform infrared (FTIR) spectra of the catalyst showed bending vibrations of the Fe-O. The X-ray diffraction (XRD) patterns of the catalyst showed characteristic diffraction peaks of α-Fe O , γ-Fe O and MnO. A four factor central composite design (CCD) coupled with response surface methodology (RSM) was applied to evaluate and optimize the important variables (catalyst addition, hydrogen peroxide dosage, initial pH value and initial dye concentration). When the reaction conditions were catalyst dosage= 0.4 g, [H O ]= 0.3 mL, pH= 2.5, [reactive brilliant blue] = 50 mg·L , and volume of solution= 500 mL at room temperature, the decolorization efficiency of reactive brilliant blue was 91.98% within 60 min. Moreover, the Fe-Mn-sepiolite catalyst had good stability for the degradation of reactive brilliant blue even after six cycles. Leaching of iron ions (<0.4 mg·L ) was observed. The decoloring process was reactive brilliant blue specific via a redox reaction. The benzene ring and naphthalene ring were first oxidized to open ring; these were then oxidized to the alcohol and carboxylic acid. The reactive brilliant blue was decomposed mainly by the attack of ·OH radicals including surface-bound ·OH radicals generated on the catalyst surface.

关键词： Fe-Mn-sepiolite catalyst     heterogeneous Fenton-like     reactive brilliant blue     homogeneous precipitation method     hydroxyl radical    

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Combining extractive heterogeneous-azeotropic distillation and hydrophilic pervaporation for enhanced

Eniko Haaz, Botond Szilagyi, Daniel Fozer, Andras Jozsef Toth

《化学科学与工程前沿（英文）》 2020年 第14卷 第5期   页码 913-927 doi: 10.1007/s11705-019-1877-1

摘要： The separation of non-ideal mixtures using distillation can be an extremely complex process and there continues to be a need to further improve these techniques. A new method which combines extractive heterogeneous-azeotropic distillation (EHAD) and hydrophilic pervaporation (HPV) for the separation of non-ideal ternary mixtures is demonstrated. This improved distillation method combines the benefits of heterogeneous-azeotropic and extractive distillations in one column but no added materials are needed as is usually the case with pervaporation. The separation of water-methanol-ethyl acetate and water-methanol-isopropyl acetate mixtures were investigated to demonstrate the accuracy of the combined EHAD/HPV technique. There is not currently an established treatment strategy for the separation of the second mixtures in the literature. These separation processes were rigorously modelled and optimized using a professional flowsheet. The objective functions were total cost and energy consumption and heat integration was also investigated. The verification of the process modelling was carried out using laboratory-scale measurements. Extractive heterogeneous-distillation combined with methanol dehydration was found to be more efficient than conventional distillation for the separation of these highly non-ideal mixtures.

关键词： hydrophilic pervaporation     non-ideal mixture     modelling     extractive heterogeneous-azeotropic distillation     heat integration    

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Heterogeneous reaction mechanism of gaseous HNO

Nan ZHAO,Qingzhu ZHANG,Wenxing WANG

《环境科学与工程前沿（英文）》 2016年 第10卷 第5期 doi: 10.1007/s11783-016-0836-z

摘要： We studied the heterogeneous reaction mechanism of gaseous HNO with solid NaCl. HCl is released from heterogeneous reactions between gaseous HNO and solid NaCl. Water molecules induce surface reconstruction of NaCl to facilitate the reaction. Sea salt particles containing NaCl are among the most abundant particulate masses in coastal atmosphere. Reactions involving sea salt particles potentially generate Cl radicals, which are released into coastal atmosphere. Cl radicals play an important role in the nitrogen and O cycles, sulfur chemistry and particle formation in the troposphere of the polluted coastal regions. This paper aimed at the heterogeneous reaction between gaseous HNO and solid NaCl. The mechanism was investigated by density functional theory (DFT). The results imply that water molecules induce the surface reconstruction, which is essential for the heterogeneous reaction. The surface reconstruction on the defective (710) surface has a barrier of 10.24 kcal·mol and is endothermic by 9.69 kcal·mol , whereas the reconstruction on the clean (100) surface has a barrier of 18.46 kcal·mol and is endothermic by 12.96 kcal·mol . The surface reconstruction involved in water-adsorbed (710) surface is more energetically favorable. In comparison, water molecules adsorbed on NaCl (100) surface likely undergo water diffusion or desorption. Further, it reveals that the coordination number of the Cl is reduced after the surface reconstruction, which assists Cl to accept the proton from HNO . HCl is released from heterogeneous reactions between gaseous HNO and solid NaCl and can react with OH free radicals to produce atomic Cl radicals. The results will offer further insights into the impact of gaseous HNO on the air quality of the coastal areas.

关键词： Seasalt particles     NaCl     HNO3     Heterogeneous reaction     Reaction mechanism     Density functional theory    

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标题 作者 时间 类型 操作

Chemical probe systems for assessing liquid–liquid mixing efficiencies of reactors

期刊论文

Energy-aware scheduling with reconstruction and frequency equalization on heterogeneous systems

Yong-xing LIU,Ken-li LI,Zhuo TANG,Ke-qin LI

期刊论文

基于分布式事件触发策略的异构非线性多智能体系统包含控制

孙雅妮,邹文成,郭健,向峥嵘

期刊论文

针对异构隐式反馈的置信度估计方法

Jing WANG, Lan-fen LIN, Heng ZHANG, Jia-qi TU, Peng-hua YU

期刊论文

Computational design of heterogeneous catalysts and gas separation materials for advanced chemical processing

Huaiwei Shi, Teng Zhou

期刊论文

Application of heterogeneous catalysis to biodiesel synthesis using microalgae oil

期刊论文

Undrained seismic bearing capacity of strip footing adjacent to a heterogeneous excavation

期刊论文

Precursor-driven structural tailoring of iron oxychloride for enhanced heterogeneous Fenton activity

期刊论文

of herding behavior of tradable green certificate market players on market efficiency: Insights from heterogeneous

期刊论文

Using heterogeneous patent network features to rank and discover influential inventors

Yong-ping DU,Chang-qing YAO,Nan LI

期刊论文

Elastic analysis of heterogeneous thick-walled spherical pressure vessels with parabolic varying properties

Keyhan KARAMI, Majid ABEDI, Mohammad ZAMANI NEJAD, Mohammad Hassan LOTFIAN

期刊论文

Enhanced heterogeneous Fenton-like activity by Cu-doped BiFeO

Jie Mao, Xie Quan, Jing Wang, Cong Gao, Shuo Chen, Hongtao Yu, Yaobin Zhang

期刊论文

Fe-Mn-sepiolite as an effective heterogeneous Fenton-like catalyst for the decolorization of reactive

Chengyuan SU,Weiguang LI,Xingzhe LIU,Xiaofei HUANG,Xiaodan YU

期刊论文

Combining extractive heterogeneous-azeotropic distillation and hydrophilic pervaporation for enhanced

Eniko Haaz, Botond Szilagyi, Daniel Fozer, Andras Jozsef Toth

期刊论文

Heterogeneous reaction mechanism of gaseous HNO

Nan ZHAO,Qingzhu ZHANG,Wenxing WANG

期刊论文